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101.
B. Spagnolo S. Spezia L. Curcio N. Pizzolato A. Fiasconaro D. Valenti P. Lo Bue E. Peri S. Colazza 《The European Physical Journal B - Condensed Matter and Complex Systems》2009,69(1):133-146
We investigate the role of the colored noise in two
biological systems: (i) adults of Nezara viridula (L.)
(Heteroptera: Pentatomidae), and (ii) polymer translocation. In the
first system we analyze, by directionality tests, the response of
N. viridula individuals to subthreshold signals plus noise
in their mating behaviour. The percentage of insects that react to
the subthreshold signal shows a nonmonotonic behaviour,
characterized by the presence of a maximum, as a function of the
noise intensity. This is the signature of the non-dynamical
stochastic resonance phenomenon. By using a “soft” threshold model
we find that the maximum of the input-output cross correlation
occurs in the same range of noise intensity values for which the
behavioural activation of the insects has a maximum. Moreover this
maximum value is lowered and shifted towards higher noise
intensities, compared to the case of white noise. In the second
biological system the noise driven translocation of short polymers
in crowded solutions is analyzed. An improved version of the Rouse
model for a flexible polymer is adopted to mimic the molecular
dynamics by taking into account both the interactions between
adjacent monomers and the effects of a Lennard-Jones potential
between all beads. The polymer dynamics is simulated in a
two-dimensional domain by numerically solving the Langevin equations
of motion in the presence of thermal fluctuations and a colored
noise source. At low temperatures or for strong colored noise
intensities the translocation process of the polymer chain is
delayed. At low noise intensity, as the polymer length increases, we
find a nonmonotonic behaviour for the mean first translocation time
of the polymer centre of inertia. We show how colored noise
influences the motion of short polymers, by inducing two different
regimes of translocation in the dynamics of molecule transport. 相似文献
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104.
A. Fiasconaro W. Ebeling E. Gudowska-Nowak 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,65(3):403-414
We give an overview over recent studies on the model of Active Brownian Motion (ABM) coupled to reservoirs providing free
energy which may be converted into kinetic energy of motion. First, we present an introduction to a general concept of active
Brownian particles which are capable to take up energy from the source and transform part of it in order to perform various
activities. In the second part of our presentation we consider applications of ABM to ratchet systems with different forms
of differentiable potentials. Both analytical and numerical evaluations are discussed for three cases of sinusoidal, staircaselike
and Mateos ratchet potentials, also with the additional loads modelled by tilted potential structure. In addition, stochastic
character of the kinetics is investigated by considering perturbation by Gaussian white noise which is shown to be responsible
for driving the directionality of the asymptotic flux in the ratchet. This stochastically driven directionality effect is visualized as a strong nonmonotonic dependence of the statistics of the right versus left trajectories of motion
leading to a net current of particles. Possible applications of the ratchet systems to molecular motors are also briefly discussed. 相似文献
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107.
Two different hexaarylbenzenes with three pyrene and three triarylamine substituents in different positions (trigonal symmetric and asymmetric arrangement) were synthesized, and their charge-transfer states were investigated by optical spectroscopy. In these multichromophoric systems triarylamine acts as the electron donor and pyrene as the electron acceptor. A reference chromophore with only one donor-acceptor pair was also investigated. All these chromophores form charge-transfer states upon photoexcitation which relax with a moderate fluorescence quantum yield to the ground state. The compounds do not differ significantly concerning most of their fluorescence properties, which shows that the fluorescent charge-transfer state is very similar in all chromophores. This observation indicates symmetry breaking for the symmetric chromophore within fluorescence lifetime of several tens of ns. This interpretation was substantiated by fluorescence excitation anisotropy measurements in a sucrose octaacetate matrix. 相似文献
108.
In recent years, solid-state NMR spectroscopy has evolved into an important characterization tool for the study of solid catalysts and chemical processes on their surface. This interest is mainly triggered by the need of environmentally benign organic transformations (“green chemistry”), which has resulted in a large number of new catalytically active hybrid materials, which are organized on the meso- and nanoscale. Typical examples of these catalysts are supported homogeneous transition metal catalysts or transition metal nanoparticles (MNPs). Solid-state NMR spectroscopy is able to characterize both the structures of these materials and the chemical processes on the catalytic surface. This article presents recent trends both on the characterization of immobilized homogeneous transition metal catalysts and on the characterization of surface species on transition metal surfaces. 相似文献
109.
《Nuclear Physics A》1999,645(1):145-174
A new operator for pion photo- and electroproduction has been developed for nuclear applications at photon equivalent energies up to 1 GeV. The model contains Born terms, vector mesons and nucleon resonances (P33(1232), P11(1440), D13(1520), S11(1535), F15(1680), and D33(1700)). The resonance contributions are included taking into account unitarity to provide the correct phases of the pion photoproduction multipoles. The Q2 dependence of electromagnetic resonance vertices is described with appropriate form factors in the electromagnetic helicity amplitudes. Within this model we have obtained good agreement with the experimental data for pion photo- and electroproduction on the nucleon for both differential cross sections and polarization observables. The model can be used as a starting point to predict and analyze forthcoming data. 相似文献
110.